P23: Development of methodology for liquefaction for the hydrolysis pretreatment of sorghum during the biofuel production process

Sunday, August 12, 2012
Columbia Hall, Terrace Level (Washington Hilton)
Camille McAvoy, Ignatius Chen, Nikita Consul, Lina Song and Jean-François P. Hamel, Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, MA

Abstract

Sorghum, a starch-containing plant, is a potential valuable bioenergy crop because of its drought tolerance, limited growth needs, and limited use as a feedstock. Production of ethanol from sorghum needs optimization to yield a maximum amount of bioethanol at a minimum energy cost. The hydrolysis pretreatment includes liquefaction and saccharification, resulting in glucose, a substrate for fermentation. A maximized glucose yield from hydrolysis should lead to a maximized ethanol yield from the entire process.

In this work biomass concentration and hydrolysis temperature were examined, and the resultant glucose yield was determined. Initial experiments used 28% (w/v) sorghum in water in a 500-mL, three-necked reactor vessel placed directly on a hotplate. This setup produced a bottom-up heating gradient that resulted in low glucose yields. This was improved by including an oil bath that allowed temperature regulation within 1°C. Liquefaction of a 28% (w/v) aqueous sorghum slurry at 85°C, using the oil bath resulted in 26.6 g/L glucose compared to 11.8 g/L glucose, when the hotplate was used. Previous methods using the same experimental setup but without the oil bath had only a 0.062 g/g (glucose/sorghum) yield whereas the oil bath methodology yielded 0.088 g/g, an approximately 42% increase in glucose yield per batch reaction. Because each liquefaction requires approximately 81.5 kJ for a two-hour incubation at 85°C, maximizing glucose yield per batch reaction is an important task for making bioethanol production less energy intensive.